- UNTIE
- Loosen
- Verb that becomes its opopsite when you swap its third and fourth letters
- Loosen a four-in-hand
- Loosen the oxfords
- Remove, as a knot
- Free
- Loosen the brogans
- Set free
- Set loose
- Disengage shoelaces?
- Loosen laces
- Prepare for takeoff
- Solve a knotty problem?
- Remove the knots from
- De-knot
- Loosen, as laces
- Open, in a way
- Take off, as scrubs
- Free of knots
- Loosen, as sneaks
- Let loose
- Get out of a bind?
- Loosen the 72-Downs
- Release, in a way
- Make easier to remove, in a way
- What you don't have to do to a loafer
- Get ready to slip off
- Cause a knot not to be
- Loosen, in a way
- Remove a knot
- Cause a knot to be not
- Loosen, as a skate
- Free from restraint
- Release from ropes
- Make a knot not
- Release
- Loosen, as a knot
- Work out the knots
- Loosen, as shoelaces
- Let loose, in a way
- Free from bondage
- Get the knots out of
- Loosen, as an ascot
- Resolve a knotty issue?
- Liberate, in a way
- Pull some strings?
- Remove, as a tether
- Disentangle
- Get the knot out
- Release a granny?
- Get the knots out
- Free, in a way
- Loosen, as a lace
- Prepare to take off, maybe
- Get the knot out of
- Remove a granny?
- Go ahead in overtime?
- Liberate from the hitching post
- Remove, as a cravat
- Free from bonds
- Loosen, as a bow
- Prepare to take off, perhaps
- Remove, as a ribbon
- Cut free from bonds
- Let free
- Open up
- Loosen a lace
- Get out of bonds
- Open, as a knot
- Open, as laces
- Open, as shoelaces
- Open, as 63 Across
- Take apart, as a knot
- Loosen the laces of
- Remove, as a rope
- Loosen up
- Loosen, as a shoe
- Loosen, as a shoelace
- Open
- Loosen, perhaps
- Opposite of "knot"
- Disconnect
- Loosen, as knots
- Open, as a 126 Across
- Loosen, as a shoelaces
- Anagram/antonym of "unite"
- Disconnect, as a rope
- Loosen, as one's laces
- Open, as 96 Across
- Prepare to remove
- Make a knot not a knot
- Prepare to remove, as shoes
- Prepare to remove, as sneakers
- Release from bondage
- Liberate, maybe
- Loose
- Open a package.
- Liberate.
- Free, as from restraint.
- Opposite of bind.
- Release from bonds
- Loosen a knot
- Loosen the bonds
- Loosen a lacet
- Loosen knots
- Remove a knot from
- Extricate
- Free from fetters
- Get rid of a knot
- Disunite
- Loosen the laces
- Pull strings?
- Ruin a bow
- Free, as knots
- Remove, as a 28-Down
- Prepare to take off?
- Loosen, as 70-Across
- Loosen, as neckwear
- Not knot?
- Leave with no strings attached?
- Get out of a tangle
- Break up, as a knot
- Remove a ribbon
- Bad Company "___ the Knot"
- Grayson Hugh "I Can't ___ You From Me"
- Release, as a buntline hitch
- Render a knot not?
- Deal with knotted laces
- Loosen Timberlands
- Destroy a knot
- Deal with a snarl
- Remove an ascot, e.g.
- Remove the tether
- Untether
- Destroy a bow
- Disentangle, e.g.
- Break a deadlock
- Correct knotted laces
- Free, as laces
- Loosen, as shoes
- De-knot laces
- Fix a knotty situation
- Remove a bow
- Free from bindings
- Free from ropes
- Liberate from restraints
- Loosen, like laces
- Opposite of "tether"
- Loosen, as a hair bow
- Prepare to take off, as skates
- Release from a knot
- Verb that becomes a family member if you add an A at the beginning
- Unfasten
- Detach
- Take off a cravat
- Remove the ropes
- Deal with a knot
- Ready the shoes for removal
- Free from restraints, in a way
- Render knotless
- Get rid of a 41-Across
- Free from a bind
- Free from a knot
- Loosen, like shoelaces
- Take a knot out of
- Loosen bonds
- Solve a knot
- Liberate from bondage
- Set free from ropes